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Aea?aeaaiee oi?aa?neoao “Euea?anueea iie?oaoi?ea”

AAA’ssE

Ethaeieea Aieiaeeie??aia

OAeE 661.715.097.

IAeA?AEAIIss A?IIAOE*IEO AOAEAAIAeI?A

OA AENIEIIEOAIIAEO EIIIIIAIO?A

EAOAE?OE*IEI IA?AOAI?AIIssI IAOOICAAIAeNUeEEO AAC?A

Niaoe?aeuei?noue 05.17.07 – o?i?/ia oaoiieia?y iaeeaa

A a o i ? a o a ? a o

aeena?oaoe?? ia caeiaoooy iaoeiaiai nooiaiy

eaiaeeaeaoa oaoi?/ieo iaoe

Euea?a-1999

Aeena?oaoe??th ? ?oeiien.

?iaioa aeeiiaia ia eaoaae?? “O?i?/ii? oaoiieia?? ia?a?iaee iaooe oa
aaco” Aea?aeaaiiai oi?aa?neoaoo “Euea?anueea iie?oaoi?ea” I?i?noa?noaa
ina?oe Oe?a?ie

Iaoeiaee ea??aiee – Caneoaeaiee ae?y/ iaoee ? oaoi?ee Oe?a?ie,

aeieoi? oaoi?/ieo iaoe, i?ioani?,

i?ia?aeiee niaoe?ae?no AAO “Aaeie” i. Ae?iaiae/,

Oaa/oe Aaneeue Onoeiiae/

Io?oe?ei? iiiiaioe – aeieoi? oaoi?/ieo iaoe,

i?ioani?, AAO “I??aia” i.Eaeoo

Oaaa? Ieeiea Aaneeueiae/

eaiaeeaeao oaoi?/ieo iaoe,

aeioeaio, i?i?aeoi? c iaa/aeueii? ?iaioe Oe?a?inueeiai

aea?aeaaiiai e?nioaoi?/iiai oi?aa?neoaoo i.Euea?a

Oooieoeueeee I?ano Iao?iae/

I?ia?aeia onoaiiaa – ?inoeooo a?ii?aai?/ii? o?i?? oa iaooio?i??,
a?aeae?e eaoae?oe/iiai neioaco, IAI Oe?a?ie, i.Ee?a.

Caoeno a?aeaoaeaoueny 25 /a?aiy 1999 ?. i 1400 aiaeei? ia
can?aeaii? niaoe?ae?ciaaii? a/aii? ?aaee Ae 35.052.07 o Aea?aeaaiiio
oi?aa?neoao? “Euea?anueea iie?oaoi?ea” (290646, Euea?a-13, ie.Na. TH?a).

C aeena?oaoe??th iiaeia iciaeiieoeny o a?ae?ioaoe? Aea?aeaaiiai
oi?aa?neoaoo “Euea?anueea iie?oaoi?ea” (Euea?a, aoe.I?ioani?nueea,1)

Aaoi?aoa?ao ?ic?neaiee 20 o?aaiy 1999 ?.

A/aiee nae?aoa?

Niaoe?ae?ciaaii? a/aii? ?aaee Ae 35.052.07.

aeieoi? o?i?/ieo iaoe
AEeciaanueeee A.I.

CAAAEUeIA OA?AEOA?ENOEEA ?IAIOE

Aeooaeuei?noue i?iaeaie. A?iiaoe/i? aoaeaaiaei?, iniaeeai aaicie, oieoie
oa eneeiee, ? aaaeeeaith ne?iaeiith aeey ?yaeo aaaaoioiiaaeieo
ae?iaieoeoa iaooio?i?/iiai neioaco. A oaia??oi?e /an c?inoa? iio?aaa a
aenieiieoaiiaeo eiiiiiaioao iioi?ieo iaeea. A?iiaoe/i? aoaeaaiaei? oa
aenieiieoaiia? eiiiiiaioe iioi?ieo iaeea a iniiaiiio iaea?aeothoue c
aaiceiiaeo o?aeoe?e oeyoii eaoae?oe/iiai ?eoi?i?iao. Oaeee i?ioean ?
neeaaeiei ? iio?aao? cia/ieo eai?oaeueieo ? aia?aaoe/ieo cao?ao.

A ca’yceo c aeao?oeeoii iaooe a Oe?a?i? aaaeeeaiai
ia?iaeii-ainiiaea?nueeiai cia/aiiy iaaoaa? i?aeaeuaiiy aoaeoeaiino?
aeei?enoaiiy iayaii? aoaeaaiaeiaai? ne?iaeie ? iiaeeea?noue cai?ie ??
aeueoa?iaoeaieie aeaea?aeaie. Oiio ?ic?iaea iiaeo i?ioean?a iaea?aeaiiy
a?iiaoe/ieo aoaeaaiaei?a oa aenieiieoaiiaeo eiiiiiaio?a iioi?ieo iaeea c
iaooicaaiaenueeeo aac?a, ye? ia caaaeaee ?aoe?iiaeueii
aeei?enoiaothoueny, ? iaaecae/aeii aeooaeueiith.

Oaiaoeea aeine?aeaeaiue ? neeaaeiaith /anoeiith iaoeiaiai iai?yieo
eaoaae?e o?i?/ii? oaoiieia? ia?a?iaee iaooe oa aaco Aea?aeaaiiai
oi?aa?neoaoo “Euea?anueea iie?oaoi?ea” – “?ic?iaea iaoeiaeo iniia
iaea?aeaiiy aenieiieoaiiaeo eiiiiiaio?a iioi?ieo iaeea,
iiaa?oiaai-aeoeaieo ?a/iaei ? aeiiii?aeieo iaoa??ae?a c iaooiai? oa
aaciai? ne?iaeie”. Iai?yi eii?aeeio?oueny iaoeiaith ?aaeith c iaooio?i??
IAI Oe?a?ie. ?iaioa aeeth/aia a Iaoe?iiaeueio iaoeiai-oaoi?/io i?ia?aio
“Iaooiia?a?iaea oa iaooio?i?y 1992-2010” (N aea?aeaaii? ?a?no?aoe??
01870095012).

Aaaeeea?noue oa aeooaeuei?noue ?iaioe i?aeoaa?aeaeo?oueny aeeth/aiiyi ??
a eii?aeeiaoe?eiee ieai I?iina?oe Oe?a?ie “Iaoeia? iniiae ?ic?iaee iiaeo
oaoiieia?e aeaeiaooeo iaooe oa aaco, aacii?iieneiaiai iaeaaeiaiiy,
iiaeeaeaii? ia?a?iaee iaooe oa aaco c iaoith iaea?aeaiiy aenieiieoaiiaeo
iioi?ieo iaeea, ianoeeueieo iaoa??ae?a, aeiiii?aeieo i?iaeoeo?a ?
iaooio?i?/ii? ne?iaeie” ca oaoiaei ni?yioaaiiyi “Iaooa ? aac Oe?a?ie” ia
ia??iae 1997 – 2001 ?iee.

Iaoa ?iaioe: ?ic?iaeoe iaoeia? iniiae oa oaoiieia?th i?ioeano
iaea?aeaiiy a?iiaoe/ieo aoaeaaiaei?a oa aenieiieoaiiaeo eiiiiiaio?a
iioi?ieo iaeea eaoae?oe/iei ia?aoai?aiiyi iaooicaaiaenueeeo aac?a ia
aenieie?aiiacaienoeo oeaie?oao oeio ZSM-5.

Iaoeiaa iiaecia: ?ic?iaeaii iiaee eaoae?caoi? – aenieie?aiiacaienoee
oeaie?o, i?iiioiaaiee aeiaeaoeaie Zn aeey i?ioeano iaea?aeaiiy
a?iiaoe/ieo aoaeaaiaei?a eaoae?oe/iei ia?aoai?aiiyi iaiane/aieo
aoaeaaiaei?a N2-N4 .

Aecia/ai? iioeiaeuei? oiiae ia?aa?ao ?aaeoe?? a?iiaoecaoe?? ia
eaoae?caoi?? OeAI+2%Zn, anoaiiaeaii, ui i?e eaoae?oe/iiio ia?aoai?aii?
aeeai?a N2-N4 aeo?ae a?iiaoe/ieo aoaeaaiaei?a noaiiaeoue ~70%.

Aia?oa anoaiiaeaii, ui eaoae?cao, iaea?aeaiee i?e eaoae?oe/iiio
ia?aoai?aii? aeeai?a N2-N4 ia oeaie?o? OeAI a iioeiaeueieo oiiaao
i?noeoue cia/io e?euee?noue ?ciaeeai?a (>70%).

Aia?oa aeine?aeaeaii aeeiai?eo eieniooai?aiiy ? anoaiiaeaii /an ?iaioe
eaoae?caoi?a (~1 aiaeeia), i?e yeiio eaoae?oe/ia aeoeai?noue oeaie?oo
i?aeoe/ii ia ci?ith?oueny.

Aia?oa aea/aii caeiiii??iino? eaoae?oe/iiai ia?aoai?aiiy
aooeeai-aooaae??iiai? o?aeoe?? (AAO) ia oeaie?o? ia?ee OeAI+2%ian.Zn.; a
iioeiaeueieo oiiaao aeo?ae a?iiaoe/ieo aoaeaaiaei?a noaiiaeoue 75%.

Anoaiiaeaia iine?aeiai?noue noaae?e ia?aoai?aiiy aeeai?a N2-N4 ia
aenieie?aiiacaienoeo oeaie?oao oeio ZSM-5, ye? i?io?eathoue ia
a?ainoaae?anueeeo (B) oa eueth?nianueeeo (L) eeneioieo oeaio?ao
eaoae?caoi?a ii ea?aii?e-eiiiiio iaoai?cio.

I?aeoe/ia cia/ei?noue ?iaioe: Aecia/aii iioeiaeuei? oiiae aeey
i?iieneiaiai cae?eniaiiy i?ioeano ia?aoai?aiiy aac?a eaoae?oe/iiai
e?ae?iao ia oeaie?oao OeAI+2%Zn oa OeAI. Iieacaii, ui io?eiaiee
eaoae?cao iiaea aooe aeei?enoaiee aeey iaea?aeaiiy ?iaeea?aeoaeueieo
a?iiaoe/ieo aoaeaaiaei?a, oa aenieiieoaiiaeo eiiiiiaio?a iioi?ieo iaeea.
Aeo?ae oe?eaaeo i?iaeoeo?a noaiiaeoue 40%ian.

Anoaiiaeaii iioeiaeuei? oiiae ia?aa?ao eaoae?oe/iiai ia?aoai?aiiy
aooeeai-aooaae??iiai? o?aeoe?? (AAO), c a?aooaaiiyi eieniooai?aiiy, oa
noai?aii iniiae oaoiieia?? aeey i?iieneiaiai cae?eniaiiy i?ioeano.

?ic?iaeaii oaoiieia?/io noaio ?aoe?iiaeueiiai aeei?enoaiiy
iaooicaaiaenueeeo aac?a, ye? a aeaiee /an aeei?enoiaothoueny ye
oaoiieia?/ia iaeeai, ui i?ecaiaeeoue aei ao?aoe iioaioe?eii aaaeeeai?
o?i?/ii? ne?iaeie oa iia??oaiith aeieia?/ii? neooaoe??.

Aoaeoeai?noue iaea?aeaieo eaoae?caoi??a ia?aa??aia a eaai?aoi??? AO
“Oe?oaoiaooa”, ui i?aeoaa?aeaeo?oueny aeoii aei?iaiaoaaiue.

Ai?iaaoe?y ?iaioe. Iniiai? iieiaeaiiy ?iaioe aeiiia?aeaeenue ia:
iaoeia?e eiioa?aioe?? AOC?a iaooi-aaciaiai i?io?eth ii i?iaeaiao
aeeaiei? ia?a?iaee iaooe (Iineaa, 1990?.); iaoeiai-i?aeoe/i?e
eiioa?aioe?? “Noai ? ia?niaeoeae ?icaeoeo iaooiia?a?iaee oa iaooio?i?? a
Oe?a?i?” (Euea?a, 1994?.); iaoeiai-i?aeoe/i?e eiioa?aioe?? OIAA (Ee?a,
1994?); iaoeiai-i?aeoe/i?e eiioa?aioe?? “Euea?anuee? o?i?/i? /eoaiiy”
(Euea?a, 1995?.); II ?a?iiaenueeiio eiia?an? ii eaoae?co “EUROPAKAT-II”
(Iaano??oo, I?aea?eaiaee, 1995?); II I?aeia?iaeiiio eiia?an? ii eaoae?co
oa aaeni?aoe?? (A?ioeeaa, Iieueoa, 1996?.); III ?a?iiaenueeiio eiia?an?
ii eaoae?co “EUROPAKAT-III” (E?ae?a, Iieueoa, 1997?.).

Ioae?eaoe??. Iniiai? ?acoeueoaoe ?iaioe iioae?eiaai? a 16 ae?oeiaaieo
?iaioao (cie?aia 6 noaoae a oaoiaeo aeo?iaeao, 2 – iaoa??aee
eiioa?aioe?e, 1- aeaiiiiaaia noaooy oa 7 – oace eiioa?aioe?e).

No?oeoo?a ? ia’?i aeena?oaoe??. Aeena?oaoe?eia ?iaioa neeaaea?oueny c
anooio, 5 ?icae?e?a, aeniiae?a, nieneo aeei?enoaieo aeaea?ae ( 133
iaeiaioaaiue) oa aeiaeaoe?a. Iaoa??aee aeeeaaeai? ia 150 noi??ieao,
i?noyoue 8 ?enoie?a oa 21 oaaeeoeth.

INIIAIEE CI?NO ?IAIOE

O ia?oiio ?icae?e? ?icaeyiooi no/aniee noai oa ia?niaeoeae ?icaeoeo
aeine?aeaeaiue a iaeano? eaoae?oe/iiai ia?aoai?aiiy aoaeaaiaeiaaeo aac?a
ia oeaie?oao oeio ZSM-5. Iaaaaeaii e?eoe/iee aiae?c eaoae?caoi??a
a?iiaoecaoe?? aeeai?a oa aeeai?a N2-N4. ?icaeyiooi iniaeeaino?
aaoa?iaaiiiai eaoae?co, ye? iia’ycai? c iaoiaeii neioaco oa
iiaeeo?eaoe?? eaoae?caoi??a ? aieeaii o?ceei-o?i?/ieo aeanoeainoae
iiaa?oi? ia eiai eaoae?oe/i? aeanoeaino?.

Ae?oaee ?icae?e i?enay/aiee iaoiaeeoe? oa aeai?o oiia aeine?aeaeaiue
eaoae?oe/iiai ia?aoai?aiiy aeeai?a N2-N4. I?iaaaeaii oa?iiaeeiai?/iee
aiae?c a?iiaoecaoe?? iaiane/aieo aoaeaaiaei?a. Anoaiiaeaii, ui ?aaeoe?th
eaoae?oe/iiai ia?aoai?aiiy aeeai?a N2-N4 c iaoith iaea?aeaiiy
a?iiaoe/ieo aoaeaaiaei?a oa?iiaeeiai?/ii iiaeeeai i?iaiaeeoe a ?ioa?aae?
oaiia?aoo? 473-1000 E. Iienaia iaoiaeeea aeine?aeaeaiiy eaoae?oe/iiai
ia?aoai?aiiy aoaeaaiaeiaaeo aac?a (i?ioi/iee iaoiae), aiae?co aeo?aeii?
ne?iaeie ? i?iaeoeo?a ?aaeoe?? (o?iiaoia?ao?/iee iaoiae) oa ?ic?aooie?a.
Aecia/aii oiiae i?iaaaeaiiy aenia?eiaioo aeey ?aae?caoe?? ?aaeeio,
aeecueeiai aei ?aaeeio ?aeaaeueiiai ?cioa?i?/iiai ?aaeoi?a.

O o?aoueiio ?icae?e? iienaii iaoiaee iaea?aeaiiy eaoae?caoi??a oa
aeine?aeaeaiiy eaoae?oe/ieo nenoai ia?aoai?aiiy aeeai?a N2-N4 a
a?iiaoe/i? aoaeaaiaei? ? aenieiieoaiia? eiiiiiaioe iioi?ieo iaeea.
Iaaaaeaii iniiai? oa?aeoa?enoeee aenieie?aiiacaienoeo oeaie?o?a OeAI oa
OeAI, ye? i?iyaeythoue aenieo aeoeai?noue oa naeaeoeai?noue a i?ioeanao
eaoae?oe/iiai ia?aoai?aiiy oa aeaioiaeythoueny a i?iieneiaiio ianooaa?.

Iienai? iaoiaee aecia/aiiy o?ceei-o?i?/ieo oa?aeoa?enoee eaoae?caoi??a.
Iaoiaeii neaiiaaii? aeaeo?iiineii?? (SEM) aeine?aeaeaii ii?oieia?th
oeaie?o?a ? aecia/aii ?ici?? e?enoae?a ca?ai eaoae?caoi??a OeAI oa OeAI.
Iaoiaeii ?aioaaiino?oeoo?iiai aiae?co (XRR) aiii?eii? oi?ie oeaie?oo
OeAI oa OeAI anoaiiaeaii, ui aiie a?aeiinyoueny aei eaoae?caoi??a oeio
ZSM-5, ?acoeueoaoe aiae?co iaaaaeai? ia ?en.1,2.

?en.1 ?aioaaiino?oeoo?iee (XRR) ?en.2
?aioaaiino?oeoo?iee (XRR)

aiae?c oeaie?o?a OeAI oa ZSM-5 aiae?c oeaie?o?a OeAI oa ZSM-5

Iaoiaeii oa?iii?ia?aiiaaii? aeani?aoe?? ai?aeo (OIAeA), anoaiiaeaii
eeneioi? aeanoeaino? aeeaieiaeaeao?iiiaaieo oeaie?o?a I-OeAI oa OeAI ?
aecia/ai? oaiia?aoo?i? iaae? i?iyao neee a?ainoaae?anueeeo (B) oa
eueth?nianueeeo (L) oeaio??a. Noia?ia eeneioi?noue eaoae?caoi?a OeAI ?
cia/ii iaioith i?ae aeey I-OeAI, iaeiae i?iyaey?oueny i?e ieae/?e
oaiia?aoo?? (?en.3,4).

Aeine?aeaeaii aieea iiaeeo?eaoi??a ia eaoae?oe/io aeoeai?noue oeaie?o?a
OeAI oa OeAI. A yeino? iiaeaeueii? aea?aii ?aaeoe?th eaoae?oe/iiai
ia?aoai?aiiy i?ii?eaio, ine?eueee oeae aoaeaaiaeaiue caeia? i?ii?aeia
iieiaeaiiy ii nai?e eaoae?oe/i?e aeoeaiino? na?aae aeeai?a N2-N4 oa
ciaoiaeeoueny a cia/ieo e?eueeinoyo a iaooicaaiaenueeeo aacao.

?en.3 OIAeA eaoae?caoi?a I-OeAI ?en.4 OIAeA eaoae?caoi?a OeAI

A ?acoeueoao? i?iaaaeaieo aeine?aeaeaiue anoaiiaeaii, ui
iiaeeo?eoaaiiy aeo?aeiiai oeaie?oo OeAI ieneaeaie iaoae?a i?ecaiaeeoue
aei cia/iiai ca?eueoaiiy aeoiaeo ??aeeiai eaoae?caoo. Ii nai?e
eaoae?oe/i?e aeoeaiino? aeine?aeaeai? iiaeeo?eaoi?e iiaeia ?ici?noeoe a
?yae: Zn > Ni > Ga > Co > Mg > Cu. Oiio aea?aii eaoae?caoi?e
iiaeeo?eiaai? Zn, ye iaea?eueo aeoeai?. Aecia/aii iioeiaeueiee ai?no
oeeieo a oeaie?o? (2%ian.) i?e yeiio aeinyaa?oueny iaeneiaeueiee aeo?ae
??aeeiai eaoae?caoo. Anoaiiaeaii, ui iayai?noue iiaeeo?eoth/i? aeiaaaee
ia aieeaa? ia eaoae?oe/io aeoeai?noue oeaie?oo OeAI.

Aecia/aii iioeiaeueio e?euee?noue ca’ycoth/iai ?-Al2O3 (30% ian.), i?e
ye?e aeinyaa?oueny aeinoaoiy aeey i?iieneiai? aenieoaoaoe?? iaoai?/ia
i?oei?noue ? caa??aa?oueny aeniea eaoae?oe/ia aeoeai?noue oeaie?o?a.
?ic?iaeaii ?aoeaioo?o oa noai?aii iniiae oaoiieia?/iiai i?ioeano
aeaioiaeaiiy eaoae?caoi??a ia i?iieneia?e onoaiiaoe? i?iaeoeoeai?noth
10o/??e.

Aeey iiaeaeueoeo aeine?aeaeaiue eaoae?oe/ieo nenoai aecia/ai? oiiae (
?ici?? ae?aiao?a ca?ia eaoae?caoi?a oa e?i?eia oaeaee?noue iioieo) i?e
yeeo eaoae?oe/ia ia?aoai?aiiy aeeai?a N2-N4 i?io?ea? o
aioo??oiueie?iaoe/i?e iaeano?.

A ?icae?e? 4 aea/aii aieea iniiaieo oaeoi??a oa aecia/aii iioeiaeuei?
oiiae eaoae?oe/iiai ia?aoai?aiiy iaiane/aieo aoaeaaiaei?a N2-N4 ia
aenieie?aiiacaienoeo oeaie?oao oeio ZSM-5. Eaoae?oe/ia ia?aoai?aiiy
aeeai?a N2-N4 ia oeaie?oao ia?ie OeAI oa OeAI+2%ian.Zn aea/aee a
?ioa?aae? oaiia?aoo? 573-873 E , ia’?iio oaeaee?noue ci?ithaaee a iaaeao
100 – 10000aiae-1.

Iniiaieie i?iaeoeoaie eaoae?oe/iiai ia?aoai?aiiy aoeeaio, i?ii?eaio,
i-aooeeaio oa aooeeai-aooaae??iiai? o?aeoe?? (AAO) ? ??aeeee eaoae?cao
oa aaciiiae?ai? i?iaeoeoe ?aaeoe??. Iaoiaeii aaci??aeeiii? o?iiaoia?ao??
anoaiiaeaii, ui eaoae?cao i?noeoue a?aie N6-N8 (aaicie, oieoie,
eneeiee), a?aie N9-N10, oa aeeaie N5-N7. Aaciiiae?ai? i?iaeoeoe
?aaeoe?? i?noyoue aiaeaiue, aeeaie N1-N5 oa aeeaie N2-N4.

?acoeueoaoe aeine?aeaeaiiy eaoae?oe/iiai ia?aoai?aiiy i?ii?eaio ia
aenieie?aiiacaienoeo oeaie?oao iaaaaeaii a oaae.1. I?e ia?aoai?aii?
N3I6 ia oeaie?o? OeAI+2%ian.Zn anoaiiaeaii, ui c? ca?eueoaiiyi

oaiia?aoo?e a?ae 573 aei 873 E nooi?iue ia?aoai?aiiy c?inoa? a?ae
88,7 aei 99,9%. Iaeneiaeueiee aeo?ae ??aeeeo aoaeaaiaei?a aeinyaa?oueny
i?e 773 E (ia’?iia oaeaee?noue 1000 aiae-1) ? noaiiaeoue 66,2%ian. C
i?aeaeuaiiyi oaiia?aoo?e aoaeaaiaei?a 70,2%.

Oaaeeoey 1

Eaoae?oe/ia ia?aoai?aiiy i?ii?eaio ia oeaie?oao oeio ZSM-5

Ia’?iia oaeae-e?noue, aiae-1 Oai-ia?a-oo?a,

E Ae-

o?ae

eaoa-

e?ca-

oo,

%ian Noo-

i?iue

ia?a-

oai-

?ai-iy

C3H6,% Neeaae aaciiiae?aieo i?iaeoeo?a, % ia. Neeaae ??aeeeo i?iaeoeo?a,
% ian. Ae-o?ae a?i-ia-oe/-ieo

aoaeaaiae-i?a,

%ian

H2 CH4 C2H6 C2H4 C3H8 C3H6 OC4 ae?-oa-oe/i? aai-cie Oieo-ie ene-eiee N9
? ae-ua

OeAI + 2% Zn

1000 573 52,9 88,7 43,1 – – 5,5 31,2 10,7 6,5 3,8 26,8 40,0 23,0 6,4
51,1

1000 673 60,7 94,6 45,5 4,7 2,3 4,9 26,3 6,9 5,6 3,4 26,0 40,0 27,3 3,3
57,2

1000 773 66,2 96,7 47,7 10,1 5,7 5,7 27,4 5,2 5,4 3,5 22,3 42,1 27,5 4,6
61,4

1000 873 61,0 99,9 57,9 15,8 7,1 3,2 22,0 1,0 0,7 5,2 20,2 42,1 27,1 5,4
64,8

10000 773 53,1 89,1 30,4 6,8 8,9 5,5 31,2 10,7 6,5 3,8 26,8 40,0 23,0
6,4 51,1

5000 773 63,2 96,7 47,7 10,1 5,7 3,1 27,1 2,9 3,4 3,2 21,7 45,9 26,1 3,1
64,0

500 773 68,4 98,8 53,2 15,1 4,8 3,2 22,0 1,0 0,7 5,2 20,2 42,1 27,1 5,4
64,8

OeAI

2000 623 64,9 97,5 25,6 0,9 4,9 6,5 39,8 9,8 12,5 69,4 9,3 3,9 6,6 10,8
30,6

1000 623 68,0 97,6 29,4 0,9 5,4 5,3 38,3 9,2 11,5 68,2 10,2 4,7 6,5 10,4
31,8

500 623 65,0 98,2 32,1 1,4 7,9 4,2 38,4 7,8 8,2 70,2 9,1 5,1 5,9 9,7
29,8

1000 573 65,4 95,2 28,1 1,0 5,2 6,3 40,0 9,3 12,1 70,8 9,3 5,0 6,3 8,6
29,2

1000 623 68,0 97,6 29,3 0,9 5,4 5,3 38,3 9,3 11,5 68,3 10,2 4,7 6,5 10,3
31,7

1000 723 60,9 98,7 29,4 2,0 6,8 7,1 37,5 8,9 8,3 65,5 13,0 7,3 9,0 5,2
34,5

?aaeoe?? a aaciiiae?aieo i?iaeoeoao ca?eueoothoueny eiioeaio?aoe??
iaoaio, aoaio, aoeeaio, oa i?iiaio ? ciaioo?oueny noia?ia eiioeaio?aoe?y
aoaeaaiaei?a N4. ??aeeee eaoae?cao, iaea?aeaiee i?e oaiia?aoo?? 573-623
E, i?noeoue cia/io e?euee?noue ae?oaoe/ieo aoaeaaiaei?a N5-N7 (~40%), c?
ca?eueoaiiyi oaiia?aoo?e a?ae 573 aei 873 E ai?no ae?oaoe/ieo
aoaeaaiaei?a ciaioo?oueny aei 4% aan. ?, a?aeiia?aeii, c?inoa? ai?no
a?iiaoe/ieo aoaeaaiaei?a.

Aieea ia’?iii? oaeaeeino? aea/aee iaaeao a?ae 100 aei 10000 aiae -1 i?e
iioeiaeuei?e oaiia?aoo?? 773 E. sse aeaeii c iaaaaeaieo aeaieo iaa?oue
i?e aenieeo ia’?iieo oaeaeeinoyo nooi?iue ia?aoai?aiiy i?ii?eaio
caeeoa?oueny aeineoue aenieei. Oae i?e W=10000 aiae -1 nooi?iue
ia?aoai?aiy i?ii?eaio noaiiaeoue 89,1%. Aeo?ae ??aeeiai eaoae?caoo
c?inoa? c? ciaioaiiyi ia’?iii? oaeaeeino? a?ae 53,1% i?e

10000 aiae -1 aei 70,2% i?e 100 aiae -1. sse aeaeii ci?ia ia’?iii?
oaeaeeino? a oe?ieiio ?ioa?aae? (a 100 ?ac) i?ecaiaeeoue aei ci?ie
aeoiaeo ??aeeiai eaoae?caoo eeoa ia 20%. Naeaeoeai?noue ooai?aiiy
a?iiaoe/ieo aoaeaaiaei?a i?e oeueiio iaeaea ia ci?ith?oueny.
Iaeneiaeueia naeaeoeai?noue ooai?aiiy a?iiaoe/ieo aoaeaaiaei?a c
i?ii?eaio ia eaoae?caoi?? OeAI+2%ian.Zn aeinyaa?oueny i?e ia’?ii?e
oaeaeeino? 1000 aiae-1 ? noaiiaeoue 66,2%. Ci?ia ia’?iii? oaeaeeino? ia
aieeaa? nooo?ai ia neeaae aaciiiae?aieo oa ??aeeeo i?iaeoeo?a.

Aeine?aeaeaiiy eaoae?oe/iiai ia?aoai?aiiy i?ii?eaio ia
iaiiaeeo?eiaaiiio eaoae?caoi?? OeAI (aeea. oaae.1) iieacaee, ui a
?ioa?aae? oaiia?aoo? 623-723 E nooi?iue ia?aoai?aiiy i?ii?eaio ? aeuei
i?ae ia eaoae?caoi?? OeAI+2%ian.Zn a aiaeia?/ieo oiiaao ? noaiiaeoue
95,2 – 99,8%. Aeo?ae ??aeeiai eaoae?caoo ciaoiaeeoueny a iaaeao 57-68%.
Iaeneiaeueia e?euee?noue ??aeeiai eaoae?caoo – 68% ooai?th?oueny i?e
oaiia?aoo?? cia/ii ieae/?e i?ae ia OeAI+2%ian.Zn. I?e iiaeaeueoiio
i?aeaeuaii? oaiia?aoo?e aeo?ae ??aeeiai eaoae?caoo aeaui ciaioo?oueny ?
i?e 773 E noaiiaeoue 57%. Eaoae?cao i?noeoue cia/io e?euee?noue
ae?oaoe/ieo aoaeaaiaei?a 67-71%, iniiaio aeieth yeiai (~ 60-70%)
neeaaeathoue aeeaie, ia?aaaaeii ?ciaoaeiae, ui aeicaiey?
aeei?enoiaoaaoe iaea?aeaiee i?iaeoeo ye aenieiieoaiiaee eiiiiiaio
iioi?ieo iaeea. A?iiaoe/ieo aoaeaaiaei?a ii??aiyii iaei, ?aooo
neeaaeathoue aeeaie oa iacia/ia e?euee?noue iaooai?a (?en.5). C
i?aeaeuaiiyi oaiia?aoo?e e?euee?noue a?iiaoe/ieo aoaeaaiaei?a a
eaoae?cao? ca?eueoo?oueny ? i?e 773 E noaiiaeoue ~35%.

?en.5 Neeaae eaoae?caoo, iaea?aeaiiai i?e eaoae?oe/iiio ia?aoai?aii?
i?ii?eaio

ia oeaie?o? OeAI (O=623 E, W=1000 aiae??)

Aieea ia’?iii? oaeaeeino? i?e eaoae?oe/iiio ia?aoai?aii? i?ii?eaio ia
eaoae?caoi?? OeAI aea/aee i?e oaiia?aoo?? 623 E. Ci?ia ia’?iii?
oaeaeeino? a aeine?aeaeoaaieo iaaeao i?aeoe/ii ia aieeaa? ia nooi?iue
ia?aoai?aiiy i?ii?eaio. Aeo?ae ??aeeiai eaoae?caoo ci?ith?oueny a
iacia/i?e i??? ? aeinyaa? iaeneiaeueiiai cia/aiiy i?e W=1000 aiae -1.
sse ? ia oeaie?o? OeAI+2%ian.Zn ?c ci?iith ia’?iii? oaeaeeino? neeaae
ooai?aieo aoaeaaiaeiaaeo aac?a oa ??aeeiai eaoae?caoo i?aeoe/ii ia
ci?iththoueny. Naeaeoeai?noue ooai?aiiy a?iiaoe/ieo aoaeaaiaei?a
ciaoiaeeoueny a iaaeao 30%, ae?oaoe/ieo aoaeaaiaei?a ~ 70%.

Oaeei /eiii, i?iaaaeai? aeine?aeaeaiiy iieacaee, ui i?e eaoae?oe/iiio
ia?aoai?aii? i?ii?eaio ia OeAI+2%ian.Zn i?e oaiia?aoo?? 773 E oa
ia’?ii?e oaeaeeino? 1000 aiae -1 aeinyaa?oueny iaeneiaeueiee aeo?ae
??aeeiai eaoae?caoo ? naeaeoeai?noue ooai?aiiy a?iiaoe/ieo aoaeaaiaei?a
(>90%). Ia eaoae?caoi?? OeAI oaiia?aoo?o 623 E oa ia’?iio oaeaee?noue
1000aiae -1 iiaeia aaaaeaoe iioeiaeueieie cia/aiiyie i?e iaea?aeaii?
eaoae?caoo, ui i?noeoue ae?oaoe/i? aoaeaaiaei?, a iniiaiiio ?ciaeeaie
(>70%). I?e ci?i? ia’?iii? oaeaeeino? a iaaeao 500-2000aiae -1 ia
aeine?aeaeoaaieo eaoae?caoi?ao aeo?ae ??aeeiai eaoae?caoo oa
naeaeoeai?noue ooai?aiiy oe?eaaeo i?iaeoeo?a ci?iththoueny ia ?noioii ?
ciaoiaeyoueny ia ??ai? iaeneiaeueiiai.

I?iaaaeaii aeine?aeaeaiiy aieeao ia?oe?aeueiiai oeneo ia eaoae?oe/ia
ia?aoai?aiiy i?ii?eaio. Aeine?aeaeaiiy iieacaee, ui ci?ia ia?oe?aeueiiai
oeneo a oe?ieeo iaaeao (4,0-274 eIa) i?aeoe/ii ia aieeaa? ia neeaae
i?iaeoeo?a ?aaeoe??. Aeey iaea?aeaiiy aenieeo aeoiae?a eaoae?caoo
i?ioean iiaeia cae?enithaaoe i?e aoiinoa?iiio aai i?aeaeuaiiio oeneo.

Aea/aii aieea iaoaio oa aiaeith, ye? i?noyoueny a cia/ieo e?eueeinoyo a
iaooicaaiaenueeeo aacao oa ? i?iaeoeoaie ?aaeoe?? ia eaoae?oe/ia
ia?aoai?aiiy N3I6 . A aeine?aeaeoaaieo oiiaao ?aaeoe?? NI4 oa I2
i?iyaeythoue naaa ye ?ia?oi? ?icaaaieee.

Aeeiai?eo eieniooai?aiiy ia aea?aieo eaoae?caoi?ao aea/aee i?e ci?i?
oaiia?aoo?e (723-823E) oa iino?ei?e ia’?ii?e oaeaeeino? (1000 aiae -1).
C? ca?eueoaiiyi /ano ?iaioe eaoae?caoi?a a?ae iaei??? aei oanoe aiaeei
nooi?iue ia?aoai?aiiy i?ii?eaio a?ae/ooii ciaioo?oueny. Oeae aieea
i?iyaey?oueny a a?eueo?e i??? c i?aeaeuaiiyi oaiia?aoo?e. Noia?ia
e?euee?noue ooai?aiiai eieno (0,22% ia i?iiouaiee i?ii?eai) ia
eaoae?caoi?? aeoaea iacia/ia ii??aiyii c i?ioeanii eaoae?oe/iiai
e?ae?iao. Ia caaaeath/e ia iacia/io e?euee?noue ooai?aiiai eieno,
aeoeai?noue eaoae?caoi?a c /anii ciaioo?oueny, oiio i?iieneiaee i?ioeano
iaiao?aeii cae?enithaaoe a ?ooiiiio oa?? eaoae?caoi?a.

Ii??aithth/e ?acoeueoaoe eaoae?oe/iiai ia?aoai?aiiy i?ii?eaio i?e
oaiia?aoo?? 773 E oa ia’?ii?e oaeaeeino? 1000aiae-1 ia aeine?aeaeoaaieo
eaoae?caoi?ao, ne?ae a?aecia/eoe, ui ye?niee neeaae iaea?aeaieo
i?iaeoeo?a nooo?ai a?ae??ciy?oueny. I?e aeei?enoaii? OeAI a ooai?aieo
aaciiiae?aieo i?iaeoeoao iaoai oa aiaeaiue i?noyoueny a cia/ii iaioeo
e?eueeinoyo, a i?iiaio oa o?aeoe?? N4 a?eueoa i?ae ia OeAI+2%ian.Zn.
Iniiaia a?aei?ii?noue i?iyao eaoae?oe/ii? ae?? aeine?aeaeoaaieo
oeaie?o?a a neeaae? ooai?aiiai ??aeeiai eaoae?caoo. Naeaeoeai?noue
ooai?aiiy a?iiaoe/ieo aoaeaaiaei?a ia OeAI+2%ian.Zn neeaaea? -66,2%, ia
OeAI -34,5%. Ii??aiyeueia oa?aeoa?enoeea naeaeoeaiino? ooai?aiiy
aoaeaaiaei?a N1 – N9+ ia aeine?aeaeoaaieo eaoae?caoi?ao iaaaaeaia ia
?en.6.

Aiae?c iaea?aeaieo ?acoeueoao?a iieacaa, ui a aeine?aeaeoaaieo oiiaao ia
eaoae?caoi?ao OeAI oa OeAI+2%ian.Zn i?io?eathoue ?aaeoe??
ie?aiia?ecaoe??, a?iiaoecaoe??, e?ae?iao aeeni?iii?oe?thaaiiy aiaeith oa
?aaeoe?? ou?eueiaiiy, ye? a iiaeaeueoiio iiaeooue i?ecaanoe aei
ooai?aiiy eieno. Iaeiae ni?aa?aeiioaiiy oa iai?yi ia?aa?ao oeeo ?aaeoe?e
??ci?. A iaeano? iecueeeo oaiia?aoo? aeine?aeaeoaai? eaoae?caoi?e
ni?eythoue ?aaeoe?yi ie?aiia?ecaoe?? ni?a?ici??ii ?c ?aaeoe?yie
a?iiaoecaoe??. A iaeano? aenieeo oaiia?aoo? ia OeAI+2%ian.Zn
i?io?eathoue ia?aaaaeii ?aaeoe?? a?iiaoecaoe??. Ia eaoae?caoi?? OeAI a
onueiio ?ioa?aae? aeine?aeaeoaaieo oaiia?aoo? ia?aaaaeathoue ?aaeoe??
ie?aiia?ecaoe??.

A aacao aeano?oeoeaieo i?ioean?a ia?a?iaee iaooe, cie?aia a aacao
eaoae?oe/iiai e?ae?iao, i?noyoueny aoeeai oa i-aooeeai (aei 20% ia., ui
ni?a?ici??ii ?c ai?noii i?ii?eaio). Aeey aeai?o iioeiaeueieo oiia i?e
noai?aii? iniia oaoiieia?? eaoae?oe/iiai ia?aoai?aiiy iaooicaaiaenueeeo
aac?a aea/aii aieea iniiaieo oaeoi??a ia ia?aoai?aiiy aooeeaio oa
aoeeaio ia aeine?aeaeoaaieo eaoae?caoi?ao. ?acoeueoaoe aeine?aeaeaiue
iaaaaeai? a oaae 2.

I?e eaoae?oe/iiio ia?aoai?aii? aooeeaio i?aeaeuaiiy oaiia?aoo?e a?ae
623 aei 823 E ca?eueoo? aeo?ae ??aeeiai eaoae?caoo a?ae 66,3 aei 71,2%
ian. Iaeneiaeueiee aeo?ae ??aeeeo aoaeaaiaei?a 71,2% aeinyaa?oueny i?e
oaiia?aoo?? 773 E. A ??aeeiio eaoae?cao? c i?aeaeuaiiyi oaiia?aoo?e
ca?eueoo?oueny e?euee?noue a?iiaoe/ieo aoaeaaiaei?a (a?ae 53,7 aei
68,8), cie?aia aeo?ae aaicieo c?inoa? a?ae 18,4 aei 35,2% ian., a
eiioeaio?aoe?y ae?oaoe/ieo aoaeaaiaei?a a?aeiia?aeii ciaioo?oueny.
Nooi?iue ia?aoai?aiiy aooeeaio a onueiio ?ioa?aae? aeine?aeaeoaaieo
oaiia?aoo? ~ 100%. C? ca?eueoaiiyi oaiia?aoo?e a ooai?aieo aacao c?inoa?
ai?no iaoaio (a?ae 7,4 aei 11,0%) oa aiaeith (a?ae 25,1 aei 38,5%) ?
ciaioo?oueny eiioeaio?aoe?y i?iiaio a?ae 38,0 aei 30,6%. Iioeiaeueiei
?ioa?aaeii oaiia?aoo? i?iaaaeaiiy i?ioeano eaoae?oe/iiai ia?aoai?aiiy
aooeeaio ia eaoae?caoi?? OeAI+2%ian.Zn ? 723-823 E i?e yeiio
aeinyaa?oueny aenieee aeo?ae ??aeeiai eaoae?caoo. I?e 773 E oa ia’?ii?e
oaeaeeino? iiaea/? aooeeaio 1000 aiae

Oaaeeoey 4

Eaoae?oe/ia ia?aoai?aiiy aeeai?a

( eaoae?caoi? OeAI, iiaeeo?eiaaiee 2% ian. oeeieo)

Ia`?i-

ia oaeae-e?noue,

aiae?? Oai-ia?a-oo?a,

E Aeo?ae

eaoa-

e?ca-

oo,

%ian. Noo-

i?iue

ia?a-

oai-

?ai-iy

Aoeeai

1000 723 60,4 95,7 47,3 8,6 12,4 4,3 21,3 1,8 3,3 12,2 22,0 38,2 23,1
4,5 53,0

1000 773 63,1 96,9 51,3 10,3 11,1 3,2 19,9 1,7 2,5 7,5 24,2 40,3 24,5
3,5 58,4

500 773 62,3 97,1 56,4 11,2 9,8 2,8 17,2 1,4 1,2 7,7 24,4 41,1 24,0 2,8
57,5

250 773 62,2 97,8 61,7 12,8 6,5 2,3 15,8 0,9 – 8,2 24,0 41,2 23,0 3,6
57,1

1000 823 61,2 97,2 57,6 11,2 9,0 3,0 18,3 0,9 – 4,9 26,4 43,7 22,9 2,1
58,2

-1 iaeneiaeueia naeaeoeai?noue ooai?aiiy a?iiaoe/ieo A ?ioa?aae?
aeine?aeaeoaaieo ia’?iieo oaeaeeinoae nooi?iue ia?aoai?aiiy aooeeaio ?
aenieei (97,5-100,0%). Neeaae aaciiiae?aieo i?iaeoeo?a oa ??aeeiai
eaoae?caoo caeeoa?oueny i?aeoe/ii iino?eiei. Iaeneiaeueiee aeo?ae
??aeeiai eaoae?caoo (71,2%) oa iaeneiaeueia naeaeoeai?noue ooai?aiiy
a?ai?a aeinyaa?oueny i?e 1000aiae -1 ? noaiiaeoue ~67,0%.

A aeine?aeaeoaaieo oiiaao i?e eaoae?oe/iiio ia?aoai?aii? aoeeaio aeo?ae
??aeeiai eaoae?caoo aeaui iaioee (~62%), i?ae i?e eaoae?oe/iiio
ia?aoai?aii? N3I6 oa N4I8. ?c i?aeaeuaiiyi oaiia?aoo?e a?ae 723 aei 823
E aeo?ae ??aeeiai eaoae?caoo ca?eueoo?oueny (a?ae 60,8 aei 63,3 % ian.).
I?e oeueiio nooi?iue ia?aoai?aiiy aoeeaio ci?ith?oueny a iaaeao
95,7-97,2%. Ci?ia ia?iii? oaeaeeino? ia aieeaa? nooo?ai ia neeaae
aaciaeo oa ??aeeeo i?iaeoeo?a. Iaeneiaeueiee aeo?ae ??aeeiai eaoae?caoo
aeinyaa?oueny i?e oaiia?aoo?? 773 E oa ia?ii?e oaeaeeino? 1000 aiae-1.

sse aeaeii c i?iaaaeaieo aeine?aeaeaiue i?e eaoae?oe/iiio ia?aoai?aii?
aooeeaio oa aoeeaio ia eaoae?caoi?? OeAI+2%ian.Zn niinoa??aathoueny o?
ae caeiiii??iino?, ui ? i?e eaoae?oe/iiio ia?aoai?aii? i?ii?eaio. Oaeei
/eiii aeey aeinyaiaiiy aenieiai aeoiaeo ??aeeiai eaoae?caoo i?e
aeinoaoiuei aenie?e naeaeoeaiino? ooai?aiiy a?iiaoe/ieo aoaeaaiaei?a
eaoae?oe/ia ia?aoai?aiiy aeeai?a N2-N4 ne?ae i?iaiaeeoe i?e
iioeiaeuei?e oaiia?aoo?? 773 E oa a ?ioa?aae? ia’?iieo
oaeaeeinoae 500-1000 aiae1.

Aooeeai-aooaae??iiaa o?aeoe?y (AAO), iaeei c iia?/ieo i?iaeoeo?a
i?ioeano i??ie?co, neeaaea?oueny c aooeeaio oa 1,3 aooaae??io (45,3 oa
54,7%ia. a?aeiia?aeii). Aeine?aeaeaiiy eaoae?oe/iiai ia?aoai?aiiy AAO ia
oeaie?o? ia?ee OeAI+2%ian.Zn iieacaee, ui nooi?iue ia?aoai?aiiy
aooeeai-aooaae??iiai? o?aeoe?? a aeine?aeaeoaaiiio ?ioa?aae? oaiia?aoo?
noaiiaeoue ~100 %, aeo?ae ??aeeiai eaoae?caoo ca?eueoo?oueny ?c
i?aeaeuaiiyi oaiia?aoo?e (oaae. 3). Iaeneiaeueiee aeo?ae ??eiai
eaoae?caoo aeinyaa?oueny i?e oaiia?aoo?? 773 E ? noaiiaeoue 76,4 % ian.,
naeaeoeai?noue ooai?aiiy a?iiaoe/ieo aoaeaaiaei?a i?e oeueiio noaiiaeoue
72,2%. sse ? i?e eaoae?oe/iiio ia?aoai?aii? aeeai?a N2-N4 c?
ca?eueoaiiyi oaiia?aoo?e a ??aeeiio eaoae?cao? c?inoa? ai?no a?ai?a
(~90%) ca ?aooiie ciaioaiiy eiioeaio?aoe?? ae?oaoe/ieo aoaeaaiaei?a. A
aeine?aeaeoaaiiio ?ioa?aae? ia’?iieo oaeaeeinoae nooi?iue ia?aoai?aiiy ?
aenieei ? iaa?oue i?e W=10000 aiae -1 noaiiaeoue 98,9%. Ci?ia ia’?iii?
oaeaeeino? i?aeoe/ii ia aieeaa? ia aeo?ae ??aeeiai eaoae?caoo
(76,5-75,5%). Iaeneiaeueiee aeo?ae ??aeeeo aoaeaaiaei?a aeinyaa?oueny
i?e ia’?ii?e oaeaeeino? 1000aiae-1, iaeiae iaa?oue i?e W=10000 aiae -1
a?i noaiiaeoue 75,2%.Ni?aa?aeiioaiiy a?iiaoe/ieo oa ae?oaoe/ieo
aoaeaaiaei?a a ??aeeiio eaoae?cao? oaea ae ye ? i?e i?e eaoae?oe/iiio
ia?aoai?aii? aeeai?a N2-N4.

Aeey aeai?o iioeiaeueieo oiia eaoae?oe/iiai ia?aoai?aiiy AAO aea/aii
aieea /ano ?iaioe eaoae?caoi?a ia ooai?aiiy eieno. Anoaiiaeaii,ui
ca?eueoaiiy /ano ?iaioe eaoae?caoi?a OeAI+2%ian.Zn i?ecaiaeeoue aei
ciaioaiiy nooiaiy ia?aoai?aiiy AAO ? ua a?eueoiai ciaioaiiy aeoiaeo
a?iiaoe/ieo aoaeaaiaei?a. Oiio aa?o/e aei oaaae a?eueoo caeaoi?noue aei
eieniooai?aiiy AAO i?ae aeeai?a, /an ia?aaoaaiiy eaoae?caoi?a a cii?
?aaeoe?? ia iiaeiai i

Oaaeeoey 3

Eaoae?oe/ia ia?aoai?aiiy aooeeai – aooaae??iiai? o?aeoe?? (AAO)

( eaoae?caoi? OeAI, iiaeeo?eiaaiee 2% ian. oeeieo)

Oaiia?aoo?a,

E Ia`-?i-

ia oaeae-e?noue,

aiae?? Aeo?ae

eaoae?ca-oo,

%ian. Nooi?iue

ia?aoai?aiiy

AAO,% Neeaae aaciiiae?aieo i?iaeoeo?a, % ia. Neeaae ??aeeeo i?iaeoeo?a,
% ian.

H2 CH4 C2H6 C2H4 C3H8 C3H6 OC4 AAO ae? -oa -oe/-i? aai -cie oieo -ie ene
-eiee N9 ?

773 1000 76,4 100,0 49,0 7,9 4,2 8,3 19,4 5,1 6,1 – 4,3 21,6 35,9 26,1
12,1

823 1000 75,4 100,0 50,0 10,4 4,8 8,1 19,2 4,5 3,0 – 3,3 20,9 39,3 26,3
10,2

773 10000 75,5 98,9 47,4 5,9 3,8 9,4 23,1 3,9 6,4 0,9 4,2 22,4 31,7 32,5
9,2

773 5000 75,8 99,2 48,1 6,2 4,0 9,3 22,4 4,0 6,0 – 4,3 22,0 31,3 30,3
12,4

773 2000 76,1 99,6 49,6 7,6 4,2 8,7 20,2 3,7 6,0 – 4,1 21,4 33,4 29,1
12,0

773 500 76,3 100,0 51,9 7,7 4,8 8,4 18,0 5,2 4,0 – 5,8 21,3 34,1 25,2
13,6

773 250 76,5 100,0 52,4 9,6 5,2 9,4 17,1 3,0 3,3 – 7,9 20,2 33,4 24,1
14,4

oaaoe 0,5 aiaeeie. Aeey aeinyaiaiiy iioeiaeueieo iieaciee?a i?ioean
aeioe?eueii i?iaiaeeoe i?e 10000 aiae-1

Ia iniia? aiae?co ?acoeueoao?a aenia?eiaioaeueieo aeine?aeaeaiue
i?eaaaeaieo a aeai?e ?iaio? oa e?oa?aoo?ieo aeaieo anoaiiaeaia
iine?aeiai?noue noaae?e ?aaeoe?? eaoae?oe/iiai ia?aoai?aiiy aeo?aeieo
aoaeaaiaei?a oa ooai?aieo i?ii?aeieo i?iaeoeo?a. A aeacaieo aeua oiiaao
i?io?eathoue ?aaeoe?? ie?aiia?ecaoe??, ?ciia?ecaoe??, e?ae?iao,
aeeni?iii?oe?iioaaiiy aiaeith, oeeee?caoe?? oa a?iiaoecaoe??.
Aeuaia?a/eneai? ?aaeoe?? iiaeeeai oiiaii iiae?eeoe ia aea? iniiai?
noaae?? – ia?aoai?aiiy (eiiaa?n?y) aeeai?a oa ?o a?iiaoecaoe?y. Ia
ia?o?e noaae?? eaoae?oe/iiai ia?aoai?aiiy aeeai?a iathoue i?noea
nii/aoeo a iniiaiiio i?ioeane e?ae?iao oa aeeni?iii?oe?iioaaiiy, ? ye
?acoeueoao ooai?ththoueny N2-N4 aeeaie. ?o eiioeaio?aoe?y caeaaeeoue
o?eueee a?ae oaiia?aoo?e ?aaeoe?? ? ia caeaaeeoue a?ae i?e?iaee
?aaaoth/iai aeeaio. Ooai?ai? aeeaie iio?i iiaeooue i?aeaeaaaoeny
aeeia?ecaoe??, /e ie?aiia?ecaoe??, ye? i?ecaiaeyoue aei ooai?aiiy
ae?oaoe/ieo niieoe N5-N7. Aeeia?i?, /e ie?aiia?i? i?ii?aei? niieoee
?aaaoth/eo aeeai?a oaeiae iiaeooue ?iciaaeaoeny, ui iiynith? a?aeiinii
iecuee? eiioeaio?aoe?? aeeia??a oa o?eia??a a ??aeeiio
eaoae?cao?.Noaae?y a?iiaoecaoe?? aeeth/a? oeeee?caoe?th ae??i?a c
iiaeeeaith ?o ?ciia?ecaoe??th, noaae?th ia?a?iciiae?eo aiaeith c
e?ioeaaei ooai?aiiyi a?ai?a. Ia i?ioean ooai?aiiy a?iiaoe/ieo niieoe
iathoue cia/iee aieea aeae?eueea iine?aeiaieo noaae?e
aeaa?ae?iaai?caoe?? oeeeeiaeeai?a oa oeeeeiae??i?a. Iaeaea? noaae??
i?io?eathoue ia eeneioieo (L) oa (B) oeaio?ao eaoae?caoi?a ii
ea?aii?e-eiiiiio iaoai?cio. Ooai?aiiy ea?aii?e-?iio ia eaoae?caoi??
OeAI+2%Zn ? ae??oaeueiei iiiaioii i?e eaoae?oe/iiio ia?aoai?aii? aeeai?a
a a?iiaoe/i? niieoee. Ea?aii?e-?ii aeeaio iiaea eaaei ia?aoai?eoenue a
oeeeeiaeeai oa oeeeeiae??i a ?acoeueoao? oeeee?caoe??. Eeneioia ooieoe?y
eaoae?caoi?a i?enei?th? oe? ?aaeoe??, ui i?aeoaa?aeaeo?oueny a?aeiinii
??aiei ni?aa?aeiioaiiyi eiioeaio?aoe?e ae?oaoe/ieo niieoe N5-N7 ?
neeaaeo ooai?aieo aac?a ?aaeoe?? i?e ia?aoai?aii? aoeeaio, i?ii?eaio oa
aooeeaio.

Ioaea eaoae?oe/ia ia?aoai?aiiy aeeai?a N2-N4 ia aenieie?aiiacaienoeo
eaoae?caoi?ao – oea eiiieaenia aaoa?iaaiia ?aaeoe?y, yea aeeth/a? a naaa
aaaaoi ie?aieo ?aaeoe?e (?aaeoe?e ie?aieo eiiiiiaio?a) ? ua a?eueoa
o?i?/ieo ?aaeoe?e, aea iaeei ? oie aea eiiiiiaio iiaea i?eeiyoe o/anoue
a aaaaoueio ?aaeoe?yo.

A i’yoiio ?icae?e? ?icaeyioo? oaoiieia?/i? aniaeoe iaea?aeaiiy
a?iiaoe/ieo aoaeaaiaei?a oa aenieiieoaiiaeo eiiiiiaio?a iioi?ieo
iaeea i?e eaoae?oe/iiio ia?aoai?aii? iaooicaaiaenueeeo aac?a ia
oeaie?oao ia?ie OeAI+2%ian.Zn oa OeAI.

?ic?aoiaaii iaoa??aeueiee aaeain i?ioeano eaoae?oe/iiai ia?aoai?aiiy
aac?a onoaiiaee eaoae?oe/iiai e?ae?iao AO “Oe?oaoiaooa” oa cai?iiiiiaaii
i?eioeeiiao oaoiieia?/io noaio. (?en.7). Aeo?aeia ne?iaeia (I) – aac
i?ioeano eaoae?oe/iiai e?ae?iao iinooia? a i?aeo?oaiee i?ino??
oaieiiai?iiee?a O-1,2, ? iiaea?oueny a o?oa/aoo i?/ I-1. Iaa??oee aac c
ci??aeea ia/? I-1 iinooia? a ?aaeoi?ii-?aaaia?aoi?iee aeie c ?ooiiei
oa?ii eaoae?caoi?a. ?aaeoi?ii-?aaaia?aoi?iee aeie neeaaea?oueny c
?aaeoi?a ? caiiaiaiiai eaoae?caoi?ii OeAI+2%Zn, aea a?aeaoaa?oueny
i?ioean eaoae?oe/iiai ia?aoai?aiiy aoaeaaiaeiaaeo aac?a oa ?aaaia?aoi?a
?A, a yeee ii eaoae?caoi?ii?iaiaeao iinooia? caeieniaaiee eaoae?caoi?.
?aaeoe?eia noi?o iinooia? a ae?ao?aaiiaee ci?ooaa/ C, aea ca ?aooiie
/anoeiaiai aeia?iaoaaiiy eiiaeainaoo, yeee iinooia? c naia?aoi?a N-1,
a?aeaoaa?oueny ?? ioieiaeaeaiiy. Aacii?iaeoeoiaa noi?o iinooia? a
o?oaiee i?ino?? oaieiiai?iiee?a O-1, O-2, aea iaa??aa? aeo?aeio
ne?iaeio, ioieiaeaeoth/enue i?e oeueiio. Aeae? aiia ioieiaeaeo?oueny a
aia?ao? iia?o?yiiai ioieiaeaeaiiy O-1 oa aiaeyiiio oieiaeeeueieeo O-2.
??aeeee eaoae?cao a?aeae?ey?oueny a?ae aaciai? oace a
aacinaia?aoi?? N-1. *anoeia

?en. 8.I?eioeeiiaa oaoiieia?/ia noaia iaea?aeaiiy a?iiaoe/ieo
aoaeaaiaei?a oa aenieiieoaiiaeo eiiiiiaio?a iioi?ieo iaeea c aac?a
eaoae?oe/iiai e?ae?iao.

eaoae?caoo nea?iao?oueny o ci?ooaa/ C. Aaeainiaa e?euee?noue eaoae?caoo
i?ioiaeeoue /a?ac ?aaeoeoe?eiee eeaiai E-1 ? iinooia? a aacinaia?aoi?
N-2. Aeae? ??aeeee eaoae?cao, yeee a iniiaiiio neeaaea?oueny c
a?iiaoe/ieo aoaeaaiaei?a N6-N9 iinooia? a ?ii?noue A-1. Aaciaa oaca c
naia?aoi?a N-1, ui i?noeoue cia/io e?euee?noue a?iiaoe/ieo aoaeaaiaei?a,
ye? ia neiiaeainoaaeeny a N-1, iinooia? a aani?aa?, yeee c?ioo?oueny
aani?aaioii (VI). Neiiaeainiaai? ia?e /a?ac naia?aoi? N-3 iinooiathoue a
oieiaeeeueiee O-4 ? a?iiaoe/i? aoaeaaiaei? (III) cae?athoueny a ?iiino?
A-1, c yei? iiaeathoueny a ?aca?aoa?iee ia?e. Caa?oo naia?aoi??a N-2 oa
N-3 oa aani?aa?a A ooai?ai? aoaeaaiaeiaa? aace N1-N4 (V) iiaeathoueny a
iaeeaio ia?aaeo. ?aaaia?iaaiee aani?aaio cieco aeani?aa?a c aeiiiiiaith
iiiie iiaea?oueny /a?ac oaieiiai?iiee O-3 ? oieiaeeeueiee O-3, ?
nea?iao?oueny ia aa?o aani?aa?a. Aeey a?aeiiaeaiiy aeoeaiino?
i?iaiaeeoueny ?aaaia?aoe?y eaoae?caoi?a oeyoii aeiaethaaiiy eieno
?aaaia?aoe?eiei aacii – noi?o iia?o?y c acioii -(IV). Caeieniaaiee
eaoae?caoi? ?c ?aaeoi?a ? iinooia? a ?aaaia?aoi? ?A, eoaee iiaea?oueny
eeniaai?niee ?aaaia?aoe?eiee aac (IV) aeey ieenethaaeueii? ?aaaia?aoe??.
A ?aaaia?aoi?? ?A a?aeaoaa?oueny aeiaethaaiiy eieno c iiaa?oi?
eaoae?caoi?a ? na?aeee eaoae?caoi? iinooia? a ?aaeoi? ?, a aace
?aaaia?aoe?? (II) aeaiaeyoueny c ?aaaia?aoi?a ?A.

AENIIAEE

?ic?iaeaii iaoeia? iniiae oa oaoiieia?th i?ioeano iaea?aeaiiy
a?iiaoe/ieo aoaeaaiaei?a oa aenieiieoaiiaeo eiiiiiaio?a iioi?ieo iaeea
eaoae?oe/iei ia?aoai?aiiyi iaooicaaiaenueeeo aac?a ia
aenieie?aiiacaienoeo oeaie?oao OeAI oa OeAI+2%ian.Zn.

?ic?iaeaii ?aoeaioo?o i?eaiooaaiiy eaoae?caoi??a ia iniia?
aenieie?aiiacaienoeo oeaie?o?a, ye? aeioneathoueny a i?iieneiaiio
ianooaa?. Iaoiaeii oa?iii?ia?aiiaaii? aeani?aoe?? ai?aeo (OIAeA)
aecia/aii iayai?noue eueth?nianueeeo (L) oa a?ainoaae?anueeeo (B)
eeneioieo oeaio??a oeaie?o?a OeAI oa OeAI oa anoaiiaeaii oaiia?aoo?i?
iaae? ?o eaoae?oe/ii? aeoeaiino?.

Iieacaii, ui iiaeeo?eaoe?y oeeieii (2%ian.) eaoae?caoi?a ia iniia? OeAI
i?aeaeuo? naeaeoeai?noue ooai?aiiy a?iiaoe/ieo aoaeaaiaei?a i?e
eaoae?oe/iiio ia?aoai?aii? aeeai?a N2-N4, iiaeeo?eaoe?y oeeieii
eaoae?caoi?a OeAI ia aieeaa? ia eiai aeoeai?noue oa naeaeoeai?noue.

Aea/aii iniiai? caeiiii??iino? i?io?eaiiy ?aaeoe?? ia?aoai?aiiy aeeai?a
(aoeeaio, i?ii?eaio oa aooeeaio) ia noai?aieo eaoae?caoi?ao ia iniia?
oeaie?o?a OeAI oa OeAI a ?ioa?aae? oaiia?aoo? 573 873 E oa ia’?iieo
oaeaeeinoae 250-10000 aiae -1. Aecia/aii iioeiaeuei? oiiae iaea?aeaiiy
a?iiaoe/ieo aoaeaaiaei?a i?e eaoae?oe/iiio ia?aoai?ai? aeeai?a N2-N4 ia
OeAI+2%ian.Zn. A ?ioa?aae? oaiia?aoo? 723-823 E oa i?e ia’?iieo
oaeaeeinoyo 500-1000 aiae -1 aeo?ae eaoae?caoo noaiiaeoue 60-70%, ai?no
a?iiaoe/ieo aoaeaaiaei?a a iueiio >90%.

Aia?oa iieacaii, ui i?e eaoae?oe/iiio ia?aoai?aii? aeeai?a, (ia
i?eeeaae? i?ii?eaio) ia oeaie?o? OeAI i?e oaiia?aoo?? 623 E a ?ioa?aae?
ia’?iieo oaeaeeinoae 500-1000 aiae -1 iaea?aeaiee eaoae?cao i?noeoue
cia/io e?euee?noue ?ciaeeai?a (>70%).

Aia?oa aea/aii ?aaeoe?th eaoae?oe/iiai ia?aoai?aiiy
aooeeai-aooaae??iiai? o?aeoe??, iia?/iiai i?iaeoeoo i?ioeano i??ie?co
aoaeaaiaeiaai? ne?iaeie, iieacaii , ui a iioeiaeueieo oiiaao aeo?ae
a?iiaoe/ieo aoaeaaiaei?a noaiiaeoue 75%.

Aia?oa aeine?aeaeaii aeeiai?eo eieniooai?aiiy ? anoaiiaeaii oa?i?i
i?ia?ao eaoae?caoi?a (~1 aiaeeia), i?e yeiio aeoeai?noue oa
naeaeoeai?noue ooai?aiiy oe?eaaeo i?iaeoeo?a i?aeoe/ii ia ci?iththoueny.

Anoaiiaeaii, ui a aeine?aeaeoaaieo oiiaao i?io?eathoue ?aaeoe??
ie?aiia?ecaoe??, ?ciia?ecaoe??, e?ae?iao, aeeni?iii?oe?iioaaiiy aiaeith,
oeeee?caoe?? a?iiaoecaoe?? oa ou?eueiaiiy. Ia eaoae?caoi??
OeAI+2%ian.Zn c i?aeaeuaiiyi oaiia?aoo?e c?inoa? aeiey ?aaeoe?e
a?iiaoecaoe??. Aeeaae ?aaeoe?? a?iiaoecaoe?? ia oeaie?o? OeAI a
aeine?aeaeoaaiiio ?ioa?aae? oaiia?aoo? cia/ii iaioee i?ae ia
OeAI+2%ian.Zn. Eaoae?oe/ia ia?aoai?aiiy iaiane/aieo aoaeaaiaei?a N2-N4
ia a?nieie?aiiacaienoeo oeaie?oao i?io?ea? ia eueth?nianueeeo (L) oa
a?ainoaae?anueeeo (B) eeneioieo oeaio?ao eaoae?caoi?a ii
ea?aii?e-eiiiiio iaoai?cio.

Cai?iiiiiaaii oaoiieia?/i? noaie eaoae?oe/iiai ia?aoai?aiiy
aoaeaaiaeiaaeo aac?a eaoae?oe/iiai e?ae?iao oa aooeeai-aooaae??iiai?
o?aeoe?? onoaiiaee i??ie?co aacieeaaeo o?aeoe?e oa ?ic?aoiaaii
iaoa??aeuei? aaeaine i?ioean?a.

Iniiaiee ci?no ?iaioe aeeeaaeaii a ianooiieo ioae?eaoe?yo:

I.I.Iaoeye, E.A.Aaa’ye, TH.A.Eae?/aanueeee Eaoae?oe/ia a?iiaoecaoe?y
i?ii?eaio oa aooaio ia iiaeeo?eiaaieo aenieie?aiiacaienoeo oeaie?oao //
A?niee Euea?anueeiai iie?oaoi?/iiai ?inoeoooo: O?i?y, oaoiieia?y ?a/iaei
oa ?o canoinoaaiiy.-Euea?a.-1991.-N250.-N.122-123.

E.A.Aaa’ye E.A., Aaaaeaeaa N.N., A.O. Oaa/oe, Iao??a A.A. Iioei?caoe?y
?aaeoe?? a?iiaoecaoe?? i?ii?eaio ia iiaeeo?eiaaieo aenieie?aiiacaienoeo
oeaie?oao //- A?niee Aea?ae. oi-oo “Euea?anueea iie?oaoi?ea”: O?i?y,
oaoiieia?y ?a/iaei oa ?o canoinoaaiiy.-Euea?a.-1993. N270. -N.40-42.

E.A.Aaa’ye, N.N.Aaaaeaeaa, A.A.Iao??a Ia?aoai?aiiy aooeeai-aooaae??iiai?
o?aeoe?? ia oeaie?o? ia?ee OeAI // A?niee AeO “Euea?anueea
iie?oaoi?ea”: O?i?y, oaoiieia?y ?a/iaei oa ?o canoinoaaiiy” -1994.-N276.
-N.91-93.

E.A.Aaa’ye, ?.I.Aec?o, A.A.Ai?aeue Aieea ia?oe?aeueiiai oeneo ia
i?io?eaiiy ?aaeoe?? a?iiaoecaoe?? i?ii?eaio // A?niee AeO “EI”-“O?i?y,
oaoiieia?y ?a/iaei oa ?o canoinoaaiiy”.-Euea?a.-1995.-N285.-N.80-82.

E.A.Aaa’ye, ?.I.Aec?o, A.O.Oaa/oe, E.I.Aeoaeiee Aieea aiaeith, iaoaio
oa ?ia?oiiai ?icaaaieea ia eaoae?oe/ia ia?aoai?aiiy i?ii?eaio //A?niee
AeO “EI”-“O?i?y, oaoi. ?a/iaei oa ?o canoinoaaiiy” -Euea?a.
-1996.-N298.-N.94-96.

N.Aaaaeaeaa, E.Aaa’ye, I.Iaoeye, A.A?ouae, I.A?aoe/ae Eaoae?oe/ia
ia?aoai?aiiy aaicei?a ia oeaie?oao oeio ZSM-5 // A?niee AeO “EI”-“O?i?y,
oaoiieia?y ?a/iaei oa ?o canoinoaaiiy” -Euea?a. -1998.-N342. -N.106-109.

A.O.Oaa/oe A.O., N.N.Aaaaeaeaa, E.I.Aeceo, O.E.E?oiae, I.I.Iaoeye,
E.A. Aaaye. Iiaua iooe iieo/aiey iai?aaeaeueiuo e a?iiaoe/aneeo
oaeaaiaei?iaeia ec i?e?iaeiiai, iiiooiiai e iaooacaaiaeneeo aacia
//Iaoa?eaeu niaau.- eiioa?aioeee AOCia iaooa-aaciaiai i?ioeey ii
i?iaeaiai aeoaieie ia?a?aaioee iaooe.-OeIEEOYiaooaoei.-I.-1990.-N.66-72.

I.Dzikh, O.Matsyak, L.Babiak, S.Abadjiev, V.Shevchuk Catalytic
conversion of i-butane over zeolites pentasil type //The materials of II
International Conference “Catalysis an Adsorption in Fuel Processing and
Environmental Protection” -Poland.-1996. -P.75-80

E.A.Aaa’ye, Aec?o ?.I., Aaaaeaeaa N.N., A.O.Oaa/oe Eaoae?oe/ia
a?iiaoecaoe?y i?ii?eaio ia aenieie?aiiacaienoeo oeaie?oao OeAI oa OeAI
// Aeai. AeIOA Oe?a?ie. N133-Oe93.-Ee?a. -1993.-N.1-10.

A.Oaa/oe, ?.Aec?o, N.Aaaaeaeaa, I.Iaoeye, E.Aaa’ye Aeueoa?iaoeai? oeyoe
iaea?aeaiiy ieao?i?a ? a?ai?a c aoaeaaiaeiaaeo aac?a ??ciiai
iioiaeaeaiiy. // Oace iaoeiai? eiioa?aioe?y “Noai ? ia?niaeoeae ?icaeoeo
oai?/ii? iaoee oa i?iieneiaino? a Cao?aeiiio ?aa?ii? Oe?a?ie”.
-Euea?a.-1994.-N.93.

?.Aec?o , E. Aaa’ye, N.Aaaaeaeaa, A.Oaa/oe ?ic?iaea oaoiieia??
iaea?aeaiiy a?ai?a c iaooicaaiaenueeeo aac?a //Oace eiioa?aioe?? IOO
“Noai ? ia?niaeoeae ?icaeoeo iaooiia?a?iaee oa iaooio?i?? a
Oe?a?i?”.-Euea?a.-1994.-N.37.

Oaa/oe A.O., Aaaaeaeaa N.N., Aaa’ye E.A., Iaoeye I.I., Aec?o ?.I.
Oaoiieia?y iaea?aeaiiy a?ai?a c iaooicaaiaenueeeo aac?a//Oace
iaoeiai-i?aeo. eiio.”Euea?anuee? o?i?/i? /eoaiiy” i?ena’y/aia iai’yo?
aeaae. ?. Eo/a?a.-Euea?a.-1995. -N.121.

?.I.Aec?o, I.I.Iaoeye, E.A.Aaa’ye, N.N.Aaaaeaeaa, A.O.Oaa/oe Iaea?aeaiiy
aenieiieoaiiaeo eiiiiiaio?a iioi?ieo iaeueieo c noiooiueiai iaooiaiai
aaco //Oace iaoeiai-i?aeo. eiioa?aioe?? OIAA “Iaooa ? aac
Oe?a?ie”.-Euea?a.-1995.-O.2.-N.97.

?.I.Aec?o, I.I.Iaoeye, E.A.Aaa’ye, A.I. Eiaia, N.N.Aaaaeaeaa, A.O.Oaa/oe
Oaoiieia?y iaea?aeaiiy a?ai?a c iaooicaaiaenueeeo aac?a // Oace
iaoeiai-i?aeo. eiioa?aioe?? OIAA “Iaooa ? aac
Oe?a?ie”.-Euea?a.-1995.-O.2.-N.143.

I.P.Dzikh, O.M.Matsyak, L.V.Babiak, S.S.Abadjiev and V.U.Shevchuk
Aromatization of propene, butane and their mixtures in microreactor and
pilot plant // The thesis of Second European Congress on Catalysis
“EUROPACAT-II”. -Maastricht (Netherlands).-1995.-P.792-795.

L.V.Babiak, O.M.Matsyak, I.P.Dzikh, S.S.Abadjiev, V.U.Shevchuk Sequense
of steps in aromatization reaction of i-butane and propene over ZSM-5
zeolite // The Thesis of Third European Congress on Catalysis
“EUROPACAT-III” -Krakow. -1997. -P.261.

AIIOAOe?ss

Aaaye E.A. Iaea?aeaiiy a?iiaoe/ieo aoaeaaiaei?a oa aenieiioaiiaeo
eiiiiiaio?a eaoae?oe/iei ia?aoai?aiiyi iaooicaaiaenueeeo aac?a.
-?oeiien.

Aeena?oaoe?y ia caeiaoooy iaoeiaiai nooiaiy eaiaeeaeaoa oaoi?/ieo iaoe
ca niaoe?aeuei?noth 05.17.07. -oaoiieia?y ia?a?iaee iaeea. -Aea?aeaaiee
oi?aa?n?oao “Euea?anueea iie?oaoi?ea”, Euea?a, 1999.

Aeena?oaoe?y i?enay/aia ieoaiith ?ic?iaee iaoeiaeo iniia oa oaoiieia??
iaea?aeaiiy a?iiaoe/ieo aoaeaaiaei?a oa aenieiieoaiiaeo eiiiiiaio?a
iioi?ieo iaeea eaoae?oe/iei ia?aoai?aiiyi aoaeaaiaeiaaeo aac?a
aeano?oeoeaieo i?ioean?a ia?a?iaee iaooe. ?ic?iaeaii aeoeaiee oa
naeaeoeaiee eaoae?caoi? ia iniia? aenieie?aiiacaienoiai oeaie?oo OeAI
iiaeeo?eiaaiiai 2%ian.Zn ?aaeoe?? a?iiaoecaoe?? aeeai?a N2-N4.
Anoaiiaeaii iioeiaeuei? oiiae iaea?aeaiiy aenieiieoaiiaeo eiiiiiaio?a
iioi?ieo iaeea eaoae?oe/iei ia?aoai?aiiyi iaiane/aieo aoaeaaiaei?a ia
oeaie?o? OeAI. Anoaiiaeaia caeaaei?noue i?ae o?ceei-o?i?/ieie oa
eaoae?oe/ieie aeanoeainoyie aea/aieo eaoae?caoi??a, cai?iiiiiaaia
iine?aeiai?noue noaae?e i?io?eaiiy eaoae?oe/iiai ia?aoai?aiiy aeeai?a
N2-N4.

?ic?iaeaii iniiae oaoiieia?? i?ioeano iaea?aeaiiy a?iiaoe/ieo
aoaeaaiaei?a oa aenieiieoaiiaeo eiiiiiaio?a iioi?ieo iaeea eaoae?oe/iei
ia?aoai?aiiyi iaooicaaiaenueeeo aac?a.

Eeth/ia? neiaa: aeeaie, oeaie?oe, eaoae?oe/ia aeoeai?noue,
naeaeoeai?noue, a?iiaoe/i? aoaeaaiaei?, aenieiieoaiia? eiiiiiaioe.

AIIIOAOeEss

Aaaye E.A. Iieo/aiea a?iiaoe/aneeo oaeaaiaei?iaeia e aunieiioaiiauo
eiiiiiaioia eaoaeeoe/aneei i?aa?auaieai iaooacaaiaeneeo aacia.
-?oeiienue.

Aeena?oaoeey ia nieneaiea o/aiie noaiaie eaiaeeaeaoa oaoie/aneeo iaoe
ii niaoeeaeueiinoe 05.17.07. – oaoiieiaey ia?a?aaioee oiieea. –
Ainoaea?noaaiiee oieaa?neoao “Eueaeanueea iieeoaoieea”, Eueaia, 1999.

Aeenna?oaoeey iinayuaia aii?ino ?ac?aaioee iao/iuo iniia e oaoiieiaee
iieo/aiey a?iiaoe/aneeo oaeaaiaei?iaeia e aunieiieoaiiauo eiiiiiaioia
iioi?iuo oiieea eaoaeeoe/aneei i?aa?auaieai oaeaaiaei?iaeieo aacia
aeano?oeoeaiuo i?ioeannia ia?a?aaioee iaooe. ?ac?aaioea i?ioeanna
?aoeeiiaeueiiai eniieueciaaiey iaooacaaiaeneeo aacia, eioi?ua ia anaaaea
eaaeeoeoee?iaaii eniieuecothony, i?aaenoaaeyao /?acae/aeiue eioa?an.

?ac?aaioai aeoeaiue naeaeoeaiue eaoaeecaoi? ia iniiaaiee
aenieie?aiiacaienoiai oeaieeoa OeAI, aeioneaaiiai a i?iiuoeaiiii
ianooaaa, iiaeeoeoee?iaaiue 2%ian.Zn . Ii?aaeaeaiu iioeiaeueiua oneiaey
iieo/aiey a?iiaoe/aneeo oaeaaiaei?iaeia eaoaeeoe/aneei i?aa?auaieai
aeeaiia N2-N4.

Eco/ai i?ioeann eaoaeeoe/aneiai i?a?auaiey iaianeuaiuo
oaeaaiaei?iaeia ia oeaieeoa OeAI, eaoaeecao, iieo/aiue a iioeiaeueiuo
oneiaeyo ninoieo a iniiaiii ec aeeaiia ecino?iaiey e iiaeao auoue
eiieueciaai eae aunieiieoaiiaue eiiiiiaio iioi?iuo oiieea.

Ii?aaeaeaia caaeneiinoue iaaeaeo oeceei-oeie/aneeie e eaoaeeoe/aneeie
naienoaaie enneaaeoaiuo eaoaeecaoi?ia. Ii?aaeaeaia
iineaaeiaaoaeueiinoue noaaeee i?ioaeaiey ?aaeoeee i?aa?auaiey aeeaiia
N2-N4 ii ea?aiiee-eiiiiio iaoaiecio ia euethenianeeo (L) e
a?ainoaaeianeeo eeneioiuo oeaio?ao eaoaeecaoi?a OeAI+2%ian.Zn.
I?aaeeiaeaiay noaia a aeinoaoi/iie noaiaie iienuaaao ?aaeoeee
ieeaiia?ecaoeee, e?aeeiaa, ia?a?ani?aaeaeaiey aiaei?iaea, oeeeeecaoeee
e a?iiaoecaoeee.

?ic?aaioaiu iniiau oaoiieiaee i?ioeanna ieo/aiey a?iiaoe/aneeo
oaeaaiaei?iaeia e aunieiieoaiiauo eiiiiiaioia iioi?i?o oiieea
eaoaeeoe/aneei i?aa?auaieai oaeaaiaei?iaeiuo aacia eaoaeeoe/aneiai
e?aeeiaa e ie?ieeca iaooyiuo o?aeoeee.

Eeth/aaua neiaa: aeeaiu, oeaieeou, eaoaeeoe/aneay aeoeaiinoue,
naeaeoeaiinoue, a?iiaoe/aneea oaeaaiaei?iaeu, aunieiieoaiiaua
eiiiiiaiou.

SUMMARY

Babiak L.V. The aromatic hydrocarbons and high-octane components of
motor fuels receiving by catalitic conversion of oil-plants gases.
-Manuscript.

Dissertation for the award of “candidate of technical sciences” degree
on the speciality 05.17.07. – Technology of production of oil. -State
University “Lvivska Polytechnica”. Lviv.1999.

Dissertation is dedicated to the technology aromatic hydrocarbons and
high-octane components of motor fuels receiving by catalitic conversion
of oil-plants gases. Catalysts with high activity and selectivity on
the basis of high-silicate zeolite modified 2%mas.Zn was elaborated. The
relationship between the physico-chemical and catalytical properties of
the investigated catalyssts was established. The mechanism of the
catalytic conversion of alkenes N2-N4 was proposed .

The basis technology of reciving the aromatic hydrocarbons and
high-octane component of motor fuels was developed.

Key words: alkene, zeolite, catalitic activity, selectivity, aromatic
hydrocarbons, high-octane components.

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